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Pustogow, Andrej; Saito, Yohei; Löhle, Anja; Sanz Alonso, Miriam; Kawamoto, Atsushi; Dobrosavljević, Vladimir; Dressel, Martin; Fratini, Simone (, Nature Communications)null (Ed.)Abstract Landau suggested that the low-temperature properties of metals can be understood in terms of long-lived quasiparticles with all complex interactions included in Fermi-liquid parameters, such as the effective mass m ⋆ . Despite its wide applicability, electronic transport in bad or strange metals and unconventional superconductors is controversially discussed towards a possible collapse of the quasiparticle concept. Here we explore the electrodynamic response of correlated metals at half filling for varying correlation strength upon approaching a Mott insulator. We reveal persistent Fermi-liquid behavior with pronounced quadratic dependences of the optical scattering rate on temperature and frequency, along with a puzzling elastic contribution to relaxation. The strong increase of the resistivity beyond the Ioffe–Regel–Mott limit is accompanied by a ‘displaced Drude peak’ in the optical conductivity. Our results, supported by a theoretical model for the optical response, demonstrate the emergence of a bad metal from resilient quasiparticles that are subject to dynamical localization and dissolve near the Mott transition.more » « less
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Fratini, Simone; Nikolka, Mark; Salleo, Alberto; Schweicher, Guillaume; Sirringhaus, Henning (, Nature Materials)
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Jacobs, Ian E.; Lin, Yue; Huang, Yuxuan; Ren, Xinglong; Simatos, Dimitrios; Chen, Chen; Tjhe, Dion; Statz, Martin; Lai, Lianglun; Finn, Peter A.; et al (, Advanced Materials)
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